Thermal conductance of metal-diamond interfaces at high pressure

Gregory T. Hohensee, R. B. Wilson, David G. Cahill

Research output: Contribution to journalArticle

Abstract

The thermal conductance of interfaces between metals and diamond, which has a comparatively high Debye temperature, is often greater than can be accounted for by two-phonon processes. The high pressures achievable in a diamond anvil cell (DAC) can significantly extend the metal phonon density of states to higher frequencies, and can also suppress extrinsic effects by greatly stiffening interface bonding. Here we report time-domain thermoreflectance measurements of metal-diamond interface thermal conductance up to 50GPa in the DAC for Pb, Au 0.95 Pd 0.05, Pt and Al films deposited on type 1A natural [100] and type 2A synthetic [110] diamond anvils. In all cases, the thermal conductances increase weakly or saturate to similar values at high pressure. Our results suggest that anharmonic conductance at metal-diamond interfaces is controlled by partial transmission processes, where a diamond phonon that inelastically scatters at the interface absorbs or emits a metal phonon.

Original languageEnglish (US)
Article number6578
JournalNature communications
Volume6
DOIs
StatePublished - Mar 2015

Fingerprint

Diamond
Phonons
Hot Temperature
Metals
diamonds
Pressure
metals
anvils
Synthetic diamonds
Debye temperature
stiffening
cells
specific heat
Temperature

ASJC Scopus subject areas

  • Chemistry(all)
  • Biochemistry, Genetics and Molecular Biology(all)
  • Physics and Astronomy(all)

Cite this

Thermal conductance of metal-diamond interfaces at high pressure. / Hohensee, Gregory T.; Wilson, R. B.; Cahill, David G.

In: Nature communications, Vol. 6, 6578, 03.2015.

Research output: Contribution to journalArticle

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