Strain-resilient electrical functionality in thin-film metal electrodes using two-dimensional interlayers

Chullhee Cho, Pilgyu Kang, Amir Taqieddin, Yuhang Jing, Keong Yong, Jin Myung Kim, Md Farhadul Haque, Narayana R. Aluru, Sung Woo Nam

Research output: Contribution to journalArticlepeer-review

Abstract

Flexible electrodes that allow electrical conductance to be maintained during mechanical deformation are required for the development of wearable electronics. However, flexible electrodes based on metal thin films on elastomeric substrates can suffer from complete and unexpected electrical disconnection after the onset of mechanical fracture across the metal. Here we show that the strain-resilient electrical performance of thin-film metal electrodes under multimodal deformation can be enhanced by using a two-dimensional interlayer. Insertion of atomically thin interlayers—graphene, molybdenum disulfide or hexagonal boron nitride—induces continuous in-plane crack deflection in thin-film metal electrodes. This leads to unique electrical characteristics (termed electrical ductility) in which electrical resistance gradually increases with strain, creating extended regions of stable resistance. Our two-dimensional interlayer electrodes can maintain a low electrical resistance beyond a strain at which conventional metal electrodes would completely disconnect. We use the approach to create a flexible electroluminescent light-emitting device with an augmented strain-resilient electrical functionality and an early damage diagnosis capability.

Original languageEnglish (US)
Pages (from-to)126-133
Number of pages8
JournalNature Electronics
Volume4
Issue number2
DOIs
StatePublished - Feb 2021

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Instrumentation
  • Electrical and Electronic Engineering

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