TY - JOUR
T1 - Natural width of the superconducting transition in epitaxial TiN films
AU - Baeva, Elmira
AU - Kolbatova, Anna
AU - Titova, Nadezhda
AU - Saha, Soham
AU - Boltasseva, Alexandra
AU - Bogdanov, Simeon
AU - Shalaev, Vladimir M.
AU - Semenov, Alexander
AU - Goltsman, Gregory N.
AU - Khrapai, Vadim
N1 - We are grateful to I Burmistrov, A Denisov, M Feigelman, I Gornyi, E K\u00F6nig, A Levchenko, A Melnikov, D Shovkun, and A Shuvaev for fruitful discussions. This study was conducted as a part of RFBR, Project Number 19-32-60076 (development of the phenomenological model for RT broadening by magnetic impurities) and the Ministry of Science and Higher Education of the Russian Federation in the framework of the Agreement 075-11-2022-026 (sample fabrication). It was also supported by strategic project \u2018Digital Transformation: Technologies, Effectiveness, Efficiency\u2019 of Higher School of Economics development programme granted by Ministry of science and higher education of Russia \u2018Priority-2030\u2019 grant as a part of \u2018Science and Universities\u2019 national project (transport measurements and the EMT model analysis) and the Basic Research Program at the HSE University (development of the model of T-fluctuations). Purdue team acknowledges support from AFOSR Grant FA9550-20-1-0124 (growth of TiN films).
PY - 2024/10/1
Y1 - 2024/10/1
N2 - We investigate the effect of various fluctuation mechanisms on the DC resistance in superconducting (SC) devices based on epitaxial titanium nitride (TiN) films. The samples we studied show a relatively steep resistive transition (RT), with a transition width Δ T / T c ∼ 0.002 − 0.025 , depending on the film thickness (20 nm, 9 nm, and 5 nm) and device dimensions. This value is significantly broader than expected due to conventional SC fluctuations ( Δ T / T c ≪ 10 − 3 ). The shape and width of the RT can be perfectly described by the well-known effective medium theory, which allows us to understand the origin of the inhomogeneity in the SC properties of TiN films. We propose that this inhomogeneity can have both dynamic and static origins. The dynamic mechanism is associated with spontaneous fluctuations in electron temperature (T-fluctuations), while the static mechanism is due to a random spatial distribution of surface magnetic disorder (MD). Our analysis has revealed clear correlations between the transition width and material parameters as well as device size for both proposed mechanisms. While T-fluctuations may contribute significantly to the observed transition width, our findings suggest that the dominant contribution comes from the MD mechanism. Our results provide new insights into the microscopic origin of broadening of the SC transition and inhomogeneity in thin SC films.
AB - We investigate the effect of various fluctuation mechanisms on the DC resistance in superconducting (SC) devices based on epitaxial titanium nitride (TiN) films. The samples we studied show a relatively steep resistive transition (RT), with a transition width Δ T / T c ∼ 0.002 − 0.025 , depending on the film thickness (20 nm, 9 nm, and 5 nm) and device dimensions. This value is significantly broader than expected due to conventional SC fluctuations ( Δ T / T c ≪ 10 − 3 ). The shape and width of the RT can be perfectly described by the well-known effective medium theory, which allows us to understand the origin of the inhomogeneity in the SC properties of TiN films. We propose that this inhomogeneity can have both dynamic and static origins. The dynamic mechanism is associated with spontaneous fluctuations in electron temperature (T-fluctuations), while the static mechanism is due to a random spatial distribution of surface magnetic disorder (MD). Our analysis has revealed clear correlations between the transition width and material parameters as well as device size for both proposed mechanisms. While T-fluctuations may contribute significantly to the observed transition width, our findings suggest that the dominant contribution comes from the MD mechanism. Our results provide new insights into the microscopic origin of broadening of the SC transition and inhomogeneity in thin SC films.
KW - effective medium theory
KW - resistivity measurements
KW - superconducting fluctuations
KW - superconducting transition
KW - ultrathin films
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U2 - 10.1088/1361-6668/ad74a1
DO - 10.1088/1361-6668/ad74a1
M3 - Article
AN - SCOPUS:85203879986
SN - 0953-2048
VL - 37
JO - Superconductor Science and Technology
JF - Superconductor Science and Technology
IS - 10
M1 - 105017
ER -