Monitoring long-term trends in sulfate and ammonium in US precipitation: Results from the National Atmospheric Deposition Program/National Trends Network

Christopher MB Lehmann, Van C. Bowersox, Robert S. Larson, Susan M Larson

Research output: Chapter in Book/Report/Conference proceedingChapter

Abstract

Data from the National Atmospheric Deposition Program/National Trends Network (NADP/NTN) indicate significant changes have occurred in precipitation chemistry and the chemical climate in the United States (US). A Seasonal Kendall Trend (SKT) analysis shows statistically significant increases in precipitation ammonium concentrations at 64% of 159 continental US NADP/NTN sites evaluated from Winter 1985 to Fall 2004 (Dec. 1984-Nov. 2004). Sulfate decreases were widespread, with an SKT analysis indicating statistically significant decreases at 89% of sites evaluated. Ratios of chemical equivalent concentrations of ammonium to sulfate in precipitation have risen to the extent that ammonium now exceeds sulfate over more than half of the continental U.S. on a precipitation-weightedmean annual basis. These trends in the concentrations of ammonium, sulfate, and other species have been accompanied by significant decreases in the frequency of acidic precipitation (pH<5.0) in the last decade.

Original languageEnglish (US)
Title of host publicationAcid Rain - Deposition to Recovery
PublisherSpringer Netherlands
Pages59-66
Number of pages8
ISBN (Print)9781402058844
DOIs
StatePublished - Dec 1 2007

Fingerprint

atmospheric deposition
ammonium
trend analysis
sulfate
monitoring
precipitation (chemistry)
ammonium sulfate
winter
climate
trend
programme
long-term trend
chemical

Keywords

  • chemical climate
  • precipitation chemistry
  • trend analysis

ASJC Scopus subject areas

  • Environmental Science(all)
  • Earth and Planetary Sciences(all)

Cite this

Monitoring long-term trends in sulfate and ammonium in US precipitation : Results from the National Atmospheric Deposition Program/National Trends Network. / Lehmann, Christopher MB; Bowersox, Van C.; Larson, Robert S.; Larson, Susan M.

Acid Rain - Deposition to Recovery. Springer Netherlands, 2007. p. 59-66.

Research output: Chapter in Book/Report/Conference proceedingChapter

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AU - Lehmann, Christopher MB

AU - Bowersox, Van C.

AU - Larson, Robert S.

AU - Larson, Susan M

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N2 - Data from the National Atmospheric Deposition Program/National Trends Network (NADP/NTN) indicate significant changes have occurred in precipitation chemistry and the chemical climate in the United States (US). A Seasonal Kendall Trend (SKT) analysis shows statistically significant increases in precipitation ammonium concentrations at 64% of 159 continental US NADP/NTN sites evaluated from Winter 1985 to Fall 2004 (Dec. 1984-Nov. 2004). Sulfate decreases were widespread, with an SKT analysis indicating statistically significant decreases at 89% of sites evaluated. Ratios of chemical equivalent concentrations of ammonium to sulfate in precipitation have risen to the extent that ammonium now exceeds sulfate over more than half of the continental U.S. on a precipitation-weightedmean annual basis. These trends in the concentrations of ammonium, sulfate, and other species have been accompanied by significant decreases in the frequency of acidic precipitation (pH<5.0) in the last decade.

AB - Data from the National Atmospheric Deposition Program/National Trends Network (NADP/NTN) indicate significant changes have occurred in precipitation chemistry and the chemical climate in the United States (US). A Seasonal Kendall Trend (SKT) analysis shows statistically significant increases in precipitation ammonium concentrations at 64% of 159 continental US NADP/NTN sites evaluated from Winter 1985 to Fall 2004 (Dec. 1984-Nov. 2004). Sulfate decreases were widespread, with an SKT analysis indicating statistically significant decreases at 89% of sites evaluated. Ratios of chemical equivalent concentrations of ammonium to sulfate in precipitation have risen to the extent that ammonium now exceeds sulfate over more than half of the continental U.S. on a precipitation-weightedmean annual basis. These trends in the concentrations of ammonium, sulfate, and other species have been accompanied by significant decreases in the frequency of acidic precipitation (pH<5.0) in the last decade.

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KW - precipitation chemistry

KW - trend analysis

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