Femtosecond X-ray absorption spectroscopy of a light-driven spin-crossover process

C. Milne; V. T. Pham; W. Gawelda; A. E. Nahhas; R. M. Van Der Veen; S. L. Johnson; P. Beaud; G. Ingold; C. Borca; D. Grolimund; R. Abela; M. Chergui; Ch Bressler

doi:10.12693/APhysPolA.117.391

Femtosecond X-ray absorption spectroscopy of a light-driven spin-crossover process

C. Milne, V. T. Pham, W. Gawelda, A. E. Nahhas, R. M. Van Der Veen, S. L. Johnson, P. Beaud, G. Ingold, C. Borca, D. Grolimund, R. Abela, M. Chergui, Ch Bressler

Research output: Contribution to journal › Article › peer-review

Abstract

Understanding the initial steps during ultrafast molecular reactions involving large spin state changes is a vital goal in structural dynamics research. These involve knowledge of the geometric structure of the system. Ultrafast X-ray absorption spectroscopy with 50-100 picosecond time resolution establishes the geometric structure of the short-lived (τ = 0:6 ns) high spin state. Here we focus on time-resolved X-ray absorption studies with 160-200 fs temporal resolution to monitor the structural evolution in this spin-conversion process.

Original language	English (US)
Pages (from-to)	391-393
Number of pages	3
Journal	Acta Physica Polonica A
Volume	117
Issue number	2
DOIs	https://doi.org/10.12693/APhysPolA.117.391
State	Published - Feb 2010
Externally published	Yes

ASJC Scopus subject areas

General Physics and Astronomy

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abstract = "Understanding the initial steps during ultrafast molecular reactions involving large spin state changes is a vital goal in structural dynamics research. These involve knowledge of the geometric structure of the system. Ultrafast X-ray absorption spectroscopy with 50-100 picosecond time resolution establishes the geometric structure of the short-lived (τ = 0:6 ns) high spin state. Here we focus on time-resolved X-ray absorption studies with 160-200 fs temporal resolution to monitor the structural evolution in this spin-conversion process.",

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doi = "10.12693/APhysPolA.117.391",

language = "English (US)",

volume = "117",

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journal = "Acta Physica Polonica A",

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T1 - Femtosecond X-ray absorption spectroscopy of a light-driven spin-crossover process

AU - Milne, C.

AU - Pham, V. T.

AU - Gawelda, W.

AU - Nahhas, A. E.

AU - Van Der Veen, R. M.

AU - Johnson, S. L.

AU - Beaud, P.

AU - Ingold, G.

AU - Borca, C.

AU - Grolimund, D.

AU - Abela, R.

AU - Chergui, M.

AU - Bressler, Ch

PY - 2010/2

Y1 - 2010/2

N2 - Understanding the initial steps during ultrafast molecular reactions involving large spin state changes is a vital goal in structural dynamics research. These involve knowledge of the geometric structure of the system. Ultrafast X-ray absorption spectroscopy with 50-100 picosecond time resolution establishes the geometric structure of the short-lived (τ = 0:6 ns) high spin state. Here we focus on time-resolved X-ray absorption studies with 160-200 fs temporal resolution to monitor the structural evolution in this spin-conversion process.

AB - Understanding the initial steps during ultrafast molecular reactions involving large spin state changes is a vital goal in structural dynamics research. These involve knowledge of the geometric structure of the system. Ultrafast X-ray absorption spectroscopy with 50-100 picosecond time resolution establishes the geometric structure of the short-lived (τ = 0:6 ns) high spin state. Here we focus on time-resolved X-ray absorption studies with 160-200 fs temporal resolution to monitor the structural evolution in this spin-conversion process.

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Femtosecond X-ray absorption spectroscopy of a light-driven spin-crossover process

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