TY - JOUR
T1 - Extracting correlation effects from momentum-resolved electron energy loss spectroscopy
T2 - Synergistic origin of the dispersion kink in Bi2.1Sr1.9CaCu2 O8+x
AU - Huang, Edwin W.
AU - Limtragool, Kridsanaphong
AU - Setty, Chandan
AU - Husain, Ali A.
AU - Mitrano, Matteo
AU - Abbamonte, Peter
AU - Phillips, Philip W.
N1 - Publisher Copyright:
© 2021 American Physical Society.
PY - 2021/1/15
Y1 - 2021/1/15
N2 - We employ momentum-resolved electron energy loss spectroscopy (M-EELS) on Bi2.1Sr1.9CaCu2O8+x to resolve the issue of the kink feature in the electron dispersion widely observed in the cuprates. To this end, we utilize the GW approximation to relate the density response function measured in M-EELS to the self-energy, isolating contributions from phonons, electrons, and the momentum dependence of the effective interaction to the decay rates. The phononic contributions, present in the M-EELS spectra due to electron-phonon coupling, lead to kink features in the corresponding single-particle spectra at energies between 40 and 80 meV, independent of the doping level. We find that a repulsive interaction constant in momentum space is able to yield the kink attributed to phonons in ARPES. Hence, our analysis of the M-EELS spectra points to local repulsive interactions as a factor that enhances the spectroscopic signatures of electron-phonon coupling in cuprates. We conclude that the strength of the kink feature in cuprates is determined by the combined action of electron-phonon coupling and electron-electron interactions.
AB - We employ momentum-resolved electron energy loss spectroscopy (M-EELS) on Bi2.1Sr1.9CaCu2O8+x to resolve the issue of the kink feature in the electron dispersion widely observed in the cuprates. To this end, we utilize the GW approximation to relate the density response function measured in M-EELS to the self-energy, isolating contributions from phonons, electrons, and the momentum dependence of the effective interaction to the decay rates. The phononic contributions, present in the M-EELS spectra due to electron-phonon coupling, lead to kink features in the corresponding single-particle spectra at energies between 40 and 80 meV, independent of the doping level. We find that a repulsive interaction constant in momentum space is able to yield the kink attributed to phonons in ARPES. Hence, our analysis of the M-EELS spectra points to local repulsive interactions as a factor that enhances the spectroscopic signatures of electron-phonon coupling in cuprates. We conclude that the strength of the kink feature in cuprates is determined by the combined action of electron-phonon coupling and electron-electron interactions.
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U2 - 10.1103/PhysRevB.103.035121
DO - 10.1103/PhysRevB.103.035121
M3 - Article
AN - SCOPUS:85100287155
SN - 2469-9950
VL - 103
JO - Physical Review B
JF - Physical Review B
IS - 3
M1 - 035121
ER -