TY - JOUR
T1 - Evidence for a robust sign-changing s-wave order parameter in monolayer films of superconducting Fe (Se,Te)/Bi2Te3
AU - Chen, Guannan
AU - Aishwarya, Anuva
AU - Hirsbrunner, Mark R.
AU - Rodriguez, Jorge Olivares
AU - Jiao, Lin
AU - Dong, Lianyang
AU - Mason, Nadya
AU - Van Harlingen, Dale
AU - Harter, John
AU - Wilson, Stephen D.
AU - Hughes, Taylor L.
AU - Madhavan, Vidya
N1 - Funding Information:
The STM work at the University of Illinois was supported by DOE under Grant- DE-SC0022101. D.V.H, N.M, T.L.H. and M.H. were supported by the DOE “Quantum Sensing and Quantum Materials” Energy Frontier Research Center under Grant DE-SC0021238. Thin film growth was supported by the DOE “Quantum Sensing and Quantum Materials” Energy Frontier Research Center under Grant DE-SC0021238 and the Gordon and Betty Moore foundation EPiQS grant #9465 for instrumentation. V.M is a CIFAR Fellow in the Quantum Materials Program and acknowledges CIFAR for support. S.D.W., J.H., and L.D. gratefully acknowledge support via the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under award DMR-1906325. This work made use of the Illinois Campus Cluster, a computing resource that is operated by the Illinois Campus Cluster Program (ICCP) in conjunction with the National Center for Supercomputing Applications (NCSA) and which is supported by funds from the University of Illinois at Urbana-Champaign.
Funding Information:
The STM work at the University of Illinois was supported by DOE under Grant- DE-SC0022101. D.V.H, N.M, T.L.H. and M.H. were supported by the DOE “Quantum Sensing and Quantum Materials” Energy Frontier Research Center under Grant DE-SC0021238. Thin film growth was supported by the DOE “Quantum Sensing and Quantum Materials” Energy Frontier Research Center under Grant DE-SC0021238 and the Gordon and Betty Moore foundation EPiQS grant #9465 for instrumentation. V.M is a CIFAR Fellow in the Quantum Materials Program and acknowledges CIFAR for support. S.D.W., J.H., and L.D. gratefully acknowledge support via the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under award DMR-1906325. This work made use of the Illinois Campus Cluster, a computing resource that is operated by the Illinois Campus Cluster Program (ICCP) in conjunction with the National Center for Supercomputing Applications (NCSA) and which is supported by funds from the University of Illinois at Urbana-Champaign.
Publisher Copyright:
© 2022, The Author(s).
PY - 2022/12
Y1 - 2022/12
N2 - The Fe-based superconductor Fe (Se,Te) combines non-trivial topology with unconventional superconductivity and may be an ideal platform to realize exotic states such as high-order topological corner modes and Majorana modes. Thin films of Fe (Se,Te) are particularly important for device fabrication and phase sensitive transport measurements. While bulk Fe (Se,Te) has been extensively studied, the nature of the superconducting order parameter in the monolayer limit has not yet been explored. In this work, we study monolayer films of Fe (Se,Te) on Bi2Te3 with scanning tunneling spectroscopy. Monolayer Fe (Se,Te)/Bi2Te3 heterostructures host a multigap superconducting state that strongly resembles the bulk. Analysis of the phase-referenced quasiparticle interference signal reveals a sign-changing s-wave order parameter similar to the bulk as well as a unique pattern of sign changes which have not been observed in the bulk. Our work establishes monolayer Fe (Se,Te)/Bi2Te3 as a robust multi-band unconventional superconductor and sets the stage for explorations of non-trivial topology in this highly-tunable system.
AB - The Fe-based superconductor Fe (Se,Te) combines non-trivial topology with unconventional superconductivity and may be an ideal platform to realize exotic states such as high-order topological corner modes and Majorana modes. Thin films of Fe (Se,Te) are particularly important for device fabrication and phase sensitive transport measurements. While bulk Fe (Se,Te) has been extensively studied, the nature of the superconducting order parameter in the monolayer limit has not yet been explored. In this work, we study monolayer films of Fe (Se,Te) on Bi2Te3 with scanning tunneling spectroscopy. Monolayer Fe (Se,Te)/Bi2Te3 heterostructures host a multigap superconducting state that strongly resembles the bulk. Analysis of the phase-referenced quasiparticle interference signal reveals a sign-changing s-wave order parameter similar to the bulk as well as a unique pattern of sign changes which have not been observed in the bulk. Our work establishes monolayer Fe (Se,Te)/Bi2Te3 as a robust multi-band unconventional superconductor and sets the stage for explorations of non-trivial topology in this highly-tunable system.
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U2 - 10.1038/s41535-022-00513-y
DO - 10.1038/s41535-022-00513-y
M3 - Article
AN - SCOPUS:85142825778
SN - 2397-4648
VL - 7
JO - npj Quantum Materials
JF - npj Quantum Materials
IS - 1
M1 - 110
ER -