Emission factors and real-time optical properties of particles emitted from traditional wood burning cookstoves

Christoph A. Roden, Tami C. Bond, Stuart Conway, Anibal Benjamin Osorto Pinel

Research output: Contribution to journalArticlepeer-review

Abstract

It is estimated that the combustion of biofuel generates 20% of all carbonaceous aerosols, yet these particles are studied less than those of other common sources. We designed and built a portable battery-operated emission-sampling cart to measure the real-time optical properties and other emission characteristics of biofuel cookstoves. In a field study in Honduras, we measured emission factors averaging 8.5 g/kg, higher than those found in previous laboratory studies. Strong flaming events emitted very dark particles with the optical properties of black particles. The elemental carbon to total carbon ratios ranged from 0.07 to 0.64, confirming that high elemental carbon fractions can be emitted from biofuel combustion and may not be used to distinguish fossil-fuel from biofuel sources when cooking is the dominant usage. Absorption Ångström exponents, representing the dependence of absorption on wavelength, ranged from 1 (black) to 5 (yellow). Strongly absorbing particles with absorption inversely dependent on wavelength were emitted separately from particles with weak absorption and strong wavelength dependence; the latter probably contained conjugated aromatic compounds. Because combustion occurs in distinct phases, different types of carbonaceous aerosols from biofuel combustion are externally mixed at emission and may have different atmospheric fates.

Original languageEnglish (US)
Pages (from-to)6750-6757
Number of pages8
JournalEnvironmental Science and Technology
Volume40
Issue number21
DOIs
StatePublished - Nov 1 2006

ASJC Scopus subject areas

  • Chemistry(all)
  • Environmental Chemistry

Fingerprint Dive into the research topics of 'Emission factors and real-time optical properties of particles emitted from traditional wood burning cookstoves'. Together they form a unique fingerprint.

Cite this