TY - JOUR
T1 - Efficiency droop contributors in InGaN green light emitting diodes
AU - Thirasuntrakul, P.
AU - Li, J.
AU - Lee, J.
AU - Chiu, Y. C.
AU - Bayram, C.
N1 - The information, data, or work presented herein was funded in part by the Advanced Research Projects Agency-Energy (ARPA-E), U.S. Department of Energy, under OPEN Program, Award No. DE-AR0001558, in part by the U. S. Air Force Office of Scientific Research (AFOSR), under Award No. FA9550-22-1-0326, and in part by the Office of Naval Research (ONR), under Award No. N00014-23-1-2423. The views and opinions of the authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. This work was carried out in the Micro and Nanotechnology Laboratory, Electrical and Computer Engineering Building, Frederick Seitz Materials Research Laboratory Central Research Facilities, and Beckman Institute for Advanced Science and Technology, University of Illinois Urbana-Champaign, IL, USA. The authors respectfully acknowledge the valuable support from Dr. Julio Soares.
PY - 2025/5/26
Y1 - 2025/5/26
N2 - Here, efficiency droop contributors (i.e., inherent Auger-Meitner recombination, polarization-induced effects, thermal effects, and light extraction) in InGaN green light emitting diodes (LEDs) are decoupled and quantified. First, a modified ABC model is developed, and external quantum efficiency measurements are taken under constant and pulsed currents ( EQE Constant and EQE Pulsed , respectively). The LED internal quantum efficiency with and without thermal effects ( IQ E Constant ABC and IQ E Pulsed ABC , respectively) is extracted using the modified model. Then, using Raman spectroscopy, the LED junction temperature is extracted. Finally, using the optical-electrical model (OEM), the polarization- and temperature-independent LED internal quantum efficiency ( IQE OEM ) is calculated from the modified ABC model and the extracted junction temperature. By comparing external ( EQE Constant ) and the three internal quantum efficiencies ( IQ E Constant ABC , IQ E Pulsed ABC , and IQE OEM ), the impacts of inherent Auger-Meitner recombination, polarization-induced effects, thermal effects, and light extraction on the efficiency droop are decoupled and quantified. It is found that inherent Auger-Meitner recombination-induced droop is approximately 49% of the total efficiency droop in commercial green LEDs, while polarization-induced effects contribute about 35%, and thermal droop accounts for nearly 16%. These findings suggest, to quash the green gap, it is critical to search for materials and device designs with low inherent Auger-Meitner coefficients and polarization fields, respectively.
AB - Here, efficiency droop contributors (i.e., inherent Auger-Meitner recombination, polarization-induced effects, thermal effects, and light extraction) in InGaN green light emitting diodes (LEDs) are decoupled and quantified. First, a modified ABC model is developed, and external quantum efficiency measurements are taken under constant and pulsed currents ( EQE Constant and EQE Pulsed , respectively). The LED internal quantum efficiency with and without thermal effects ( IQ E Constant ABC and IQ E Pulsed ABC , respectively) is extracted using the modified model. Then, using Raman spectroscopy, the LED junction temperature is extracted. Finally, using the optical-electrical model (OEM), the polarization- and temperature-independent LED internal quantum efficiency ( IQE OEM ) is calculated from the modified ABC model and the extracted junction temperature. By comparing external ( EQE Constant ) and the three internal quantum efficiencies ( IQ E Constant ABC , IQ E Pulsed ABC , and IQE OEM ), the impacts of inherent Auger-Meitner recombination, polarization-induced effects, thermal effects, and light extraction on the efficiency droop are decoupled and quantified. It is found that inherent Auger-Meitner recombination-induced droop is approximately 49% of the total efficiency droop in commercial green LEDs, while polarization-induced effects contribute about 35%, and thermal droop accounts for nearly 16%. These findings suggest, to quash the green gap, it is critical to search for materials and device designs with low inherent Auger-Meitner coefficients and polarization fields, respectively.
UR - https://www.scopus.com/pages/publications/105006677668
UR - https://www.scopus.com/pages/publications/105006677668#tab=citedBy
U2 - 10.1063/5.0272756
DO - 10.1063/5.0272756
M3 - Article
AN - SCOPUS:105006677668
SN - 0003-6951
VL - 126
JO - Applied Physics Letters
JF - Applied Physics Letters
IS - 21
M1 - 211103
ER -