Dual-pump CARS measurements in a hydrogen diffusion flame in cross-flow with AC dielectric barrier discharge

This paper presents dual-pump coherent anti-Stokes Raman scattering (CARS) measurements for simultaneous detection of flow temperature and relative concentration, applied to the characterization of a discharge-coupled reacting jet in a cross flow. The diagnostic is hydrogen Q-branch based, providing a much wider dynamic range compared to detection in the S-branch. For a previously developed dielectric barrier discharge, aligned co-Axially with the fuel jet, OH planar laser induced fluorescence measurements show that the disturbance in the flame boundary leads to mixing enhancement. The H₂-N₂ dual-pump CARS measurement was used to map two-dimensional temperature distributions. The increase of the maximum temperature was up to 300 K, with 50% more H₂ consumption, providing the reason for the decrease in the flame length by 25%. The increase of the relative H₂O-H₂ fraction was accompanied with a temperature increase, which indicates local equivalence ratios of below 1. The H₂-O₂ dual-pump measurements confirmed that the fuel-oxidizer ratios remain in the fuel-lean side at most of the probed locations.