TY - JOUR
T1 - Combining Satellite-Derived PM2.5 Data and a Reduced-Form Air Quality Model to Support Air Quality Analysis in US Cities
AU - Gallagher, Ciaran L.
AU - Holloway, Tracey
AU - Tessum, Christopher W.
AU - Jackson, Clara M.
AU - Heck, Colleen
N1 - This study was funded by NASA Grant 80NSSC22K1678 and NASA Grant 80NSSC21K0427, as well as The Office of the Vice Chancellor for Research and Graduate Education at the University of Wisconsin–Madison. The authors thank Jenny Bratburd, Alicia Hoffman, and Lizzy Kysela for their edits and Brandon Wolf for his Python knowledge.
PY - 2023/5
Y1 - 2023/5
N2 - Air quality models can support pollution mitigation design by simulating policy scenarios and conducting source contribution analyses. The Intervention Model for Air Pollution (InMAP) is a powerful tool for equitable policy design as its variable resolution grid enables intra-urban analysis, the scale of which most environmental justice inquiries are levied. However, InMAP underestimates particulate sulfate and overestimates particulate ammonium formation, errors that limit the model's relevance to city-scale decision-making. To reduce InMAP's biases and increase its relevancy for urban-scale analysis, we calculate and apply scaling factors (SFs) based on observational data and advanced models. We consider both satellite-derived speciated PM2.5 from Washington University and ground-level monitor measurements from the U.S. Environmental Protection Agency, applied with different scaling methodologies. Relative to ground-monitor data, the unscaled InMAP model fails to meet a normalized mean bias performance goal of <±10% for most of the PM2.5 components it simulates (pSO4: −48%, pNO3: 8%, pNH4: 69%), but with city-specific SFs it achieves the goal benchmarks for every particulate species. Similarly, the normalized mean error performance goal of <35% is not met with the unscaled InMAP model (pSO4: 53%, pNO3: 52%, pNH4: 80%) but is met with the city-scaling approach (15%–27%). The city-specific scaling method also improves the R2 value from 0.11 to 0.59 (ranging across particulate species) to the range of 0.36–0.76. Scaling increases the percent pollution contribution of electric generating units (EGUs) (nationwide 4%) and non-EGU point sources (nationwide 6%) and decreases the agriculture sector's contribution (nationwide −6%).
AB - Air quality models can support pollution mitigation design by simulating policy scenarios and conducting source contribution analyses. The Intervention Model for Air Pollution (InMAP) is a powerful tool for equitable policy design as its variable resolution grid enables intra-urban analysis, the scale of which most environmental justice inquiries are levied. However, InMAP underestimates particulate sulfate and overestimates particulate ammonium formation, errors that limit the model's relevance to city-scale decision-making. To reduce InMAP's biases and increase its relevancy for urban-scale analysis, we calculate and apply scaling factors (SFs) based on observational data and advanced models. We consider both satellite-derived speciated PM2.5 from Washington University and ground-level monitor measurements from the U.S. Environmental Protection Agency, applied with different scaling methodologies. Relative to ground-monitor data, the unscaled InMAP model fails to meet a normalized mean bias performance goal of <±10% for most of the PM2.5 components it simulates (pSO4: −48%, pNO3: 8%, pNH4: 69%), but with city-specific SFs it achieves the goal benchmarks for every particulate species. Similarly, the normalized mean error performance goal of <35% is not met with the unscaled InMAP model (pSO4: 53%, pNO3: 52%, pNH4: 80%) but is met with the city-scaling approach (15%–27%). The city-specific scaling method also improves the R2 value from 0.11 to 0.59 (ranging across particulate species) to the range of 0.36–0.76. Scaling increases the percent pollution contribution of electric generating units (EGUs) (nationwide 4%) and non-EGU point sources (nationwide 6%) and decreases the agriculture sector's contribution (nationwide −6%).
KW - NAAQS
KW - decision-making
KW - environmental justice
KW - fine particulate matter
KW - reduced-form model
KW - satellite-derived PM
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U2 - 10.1029/2023GH000788
DO - 10.1029/2023GH000788
M3 - Article
C2 - 37181009
AN - SCOPUS:85160444297
SN - 2471-1403
VL - 7
JO - GeoHealth
JF - GeoHealth
IS - 5
M1 - e2023GH000788
ER -