Absence of a bulk signature of a charge density wave in hard x-ray measurements of UTe2

Caitlin S. Kengle, Dipanjan Chaudhuri, Xuefei Guo, Thomas A. Johnson, Simon Bettler, Wolfgang Simeth, Matthew J. Krogstad, Zahir Islam, Sheng Ran, Shanta R. Saha, Johnpierre Paglione, Nicholas P. Butch, Eduardo Fradkin, Vidya Madhavan, Peter Abbamonte

Research output: Contribution to journalArticlepeer-review

Abstract

The long-sought pair density wave (PDW) is an exotic phase of matter in which charge density wave (CDW) order is intertwined with the amplitude or phase of coexisting, superconducting order. Originally predicted to exist in copper-oxides, circumstantial evidence for PDW order now exists in a variety of materials. Recently, scanning tunneling microscopy (STM) studies have reported evidence for a three-component CDW at the surface of the heavy-fermion superconductor,UTe2, persisting below its superconducting transition temperature [Aishwarya, Nature 618, 928933 (2023)0028-083610.1038/s41586-023-06005-8; Gu, Nature 618, 921927 (2023)0028-083610.1038/s41586-023-05919-7; LaFleur, Nat. Commun. 15, 4456 (2024)2041-172310.1038/s41467-024-48844-7]. Here, we use hard x-ray diffraction measurements on crystals of UTe2 at T=1.9 and 12 K to search for a bulk signature of this CDW. Using STM measurements as a constraint, we calculate the expected locations of CDW superlattice peaks and sweep a large volume of reciprocal space in search of a signature. We fail to find any evidence for a CDW near any of the expected superlattice positions in many Brillouin zones. We estimate an upper bound on the CDW lattice distortion of umax?4×10-3Å. Our results suggest that the CDW observed in STM is either purely electronic, somehow lacking a signature in the lattice, or is restricted to the material surface.

Original languageEnglish (US)
Article number145101
JournalPhysical Review B
Volume110
Issue number14
DOIs
StatePublished - Oct 1 2024

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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