TY - JOUR
T1 - Absence of a bulk signature of a charge density wave in hard x-ray measurements of UTe2
AU - Kengle, Caitlin S.
AU - Chaudhuri, Dipanjan
AU - Guo, Xuefei
AU - Johnson, Thomas A.
AU - Bettler, Simon
AU - Simeth, Wolfgang
AU - Krogstad, Matthew J.
AU - Islam, Zahir
AU - Ran, Sheng
AU - Saha, Shanta R.
AU - Paglione, Johnpierre
AU - Butch, Nicholas P.
AU - Fradkin, Eduardo
AU - Madhavan, Vidya
AU - Abbamonte, Peter
N1 - Publisher Copyright:
© 2024 American Physical Society.
PY - 2024/10/1
Y1 - 2024/10/1
N2 - The long-sought pair density wave (PDW) is an exotic phase of matter in which charge density wave (CDW) order is intertwined with the amplitude or phase of coexisting, superconducting order. Originally predicted to exist in copper-oxides, circumstantial evidence for PDW order now exists in a variety of materials. Recently, scanning tunneling microscopy (STM) studies have reported evidence for a three-component CDW at the surface of the heavy-fermion superconductor,UTe2, persisting below its superconducting transition temperature [Aishwarya, Nature 618, 928933 (2023)0028-083610.1038/s41586-023-06005-8; Gu, Nature 618, 921927 (2023)0028-083610.1038/s41586-023-05919-7; LaFleur, Nat. Commun. 15, 4456 (2024)2041-172310.1038/s41467-024-48844-7]. Here, we use hard x-ray diffraction measurements on crystals of UTe2 at T=1.9 and 12 K to search for a bulk signature of this CDW. Using STM measurements as a constraint, we calculate the expected locations of CDW superlattice peaks and sweep a large volume of reciprocal space in search of a signature. We fail to find any evidence for a CDW near any of the expected superlattice positions in many Brillouin zones. We estimate an upper bound on the CDW lattice distortion of umax?4×10-3Å. Our results suggest that the CDW observed in STM is either purely electronic, somehow lacking a signature in the lattice, or is restricted to the material surface.
AB - The long-sought pair density wave (PDW) is an exotic phase of matter in which charge density wave (CDW) order is intertwined with the amplitude or phase of coexisting, superconducting order. Originally predicted to exist in copper-oxides, circumstantial evidence for PDW order now exists in a variety of materials. Recently, scanning tunneling microscopy (STM) studies have reported evidence for a three-component CDW at the surface of the heavy-fermion superconductor,UTe2, persisting below its superconducting transition temperature [Aishwarya, Nature 618, 928933 (2023)0028-083610.1038/s41586-023-06005-8; Gu, Nature 618, 921927 (2023)0028-083610.1038/s41586-023-05919-7; LaFleur, Nat. Commun. 15, 4456 (2024)2041-172310.1038/s41467-024-48844-7]. Here, we use hard x-ray diffraction measurements on crystals of UTe2 at T=1.9 and 12 K to search for a bulk signature of this CDW. Using STM measurements as a constraint, we calculate the expected locations of CDW superlattice peaks and sweep a large volume of reciprocal space in search of a signature. We fail to find any evidence for a CDW near any of the expected superlattice positions in many Brillouin zones. We estimate an upper bound on the CDW lattice distortion of umax?4×10-3Å. Our results suggest that the CDW observed in STM is either purely electronic, somehow lacking a signature in the lattice, or is restricted to the material surface.
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U2 - 10.1103/PhysRevB.110.145101
DO - 10.1103/PhysRevB.110.145101
M3 - Article
AN - SCOPUS:85206436501
SN - 2469-9950
VL - 110
JO - Physical Review B
JF - Physical Review B
IS - 14
M1 - 145101
ER -