Abstract
Lack of good ways to incorporate functional features and materials into 3D architectures has impeded progress in 3D photonic crystals (PhCs). Utilizing a modified transfer printing strategy, this study demonstrates the introduction of functional external materials of a diversity of form-factors into the interior of holographically defined 3D PhCs. PhCs containing solid SU-8 features, layers of porous silicon (PSi) or emissive LaF3:Nd3+ nanocrystals, and silica colloids are formed. For the LaF3:Nd3+ layer, both enhancement (≈50%) and suppression (≈25%) of the spontaneous emission (λ ≈ 1.32 μm) could be realized by modifying the position of the photonic crystal stop band relative to the rare earth emission. Finite-difference time-domain simulations suggest the observed spontaneous emission modification is a result of Bragg mirror-like reflection, while the measured enhancement is likely caused by the spontaneous emission coupling to a defect mode. Via electrodeposition, this study demonstrates structural inversion of a low refractive index photonic crystal (photoresist-based) to a high (Cu2O) refractive index contrast photonic crystal in the presence of an embedded defect, providing an opportunity to enhance the light-matter interactions using a materials system with transparency in the visible.
| Original language | English (US) |
|---|---|
| Pages (from-to) | 1533-1540 |
| Number of pages | 8 |
| Journal | Advanced Optical Materials |
| Volume | 4 |
| Issue number | 10 |
| DOIs | |
| State | Published - Oct 1 2016 |
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Keywords
- emission modification
- functional defects
- holographic photonic crystals
- material conversion
- transfer printing
ASJC Scopus subject areas
- Electronic, Optical and Magnetic Materials
- Atomic and Molecular Physics, and Optics
Cite this
3D Holographic Photonic Crystals Containing Embedded Functional Features. / Zhang, Runyu; Ning, Hailong; Krueger, Neil A.; Bacon-Brown, Daniel; Braun, Paul V.
In: Advanced Optical Materials, Vol. 4, No. 10, 01.10.2016, p. 1533-1540.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - 3D Holographic Photonic Crystals Containing Embedded Functional Features
AU - Zhang, Runyu
AU - Ning, Hailong
AU - Krueger, Neil A.
AU - Bacon-Brown, Daniel
AU - Braun, Paul V.
PY - 2016/10/1
Y1 - 2016/10/1
N2 - Lack of good ways to incorporate functional features and materials into 3D architectures has impeded progress in 3D photonic crystals (PhCs). Utilizing a modified transfer printing strategy, this study demonstrates the introduction of functional external materials of a diversity of form-factors into the interior of holographically defined 3D PhCs. PhCs containing solid SU-8 features, layers of porous silicon (PSi) or emissive LaF3:Nd3+ nanocrystals, and silica colloids are formed. For the LaF3:Nd3+ layer, both enhancement (≈50%) and suppression (≈25%) of the spontaneous emission (λ ≈ 1.32 μm) could be realized by modifying the position of the photonic crystal stop band relative to the rare earth emission. Finite-difference time-domain simulations suggest the observed spontaneous emission modification is a result of Bragg mirror-like reflection, while the measured enhancement is likely caused by the spontaneous emission coupling to a defect mode. Via electrodeposition, this study demonstrates structural inversion of a low refractive index photonic crystal (photoresist-based) to a high (Cu2O) refractive index contrast photonic crystal in the presence of an embedded defect, providing an opportunity to enhance the light-matter interactions using a materials system with transparency in the visible.
AB - Lack of good ways to incorporate functional features and materials into 3D architectures has impeded progress in 3D photonic crystals (PhCs). Utilizing a modified transfer printing strategy, this study demonstrates the introduction of functional external materials of a diversity of form-factors into the interior of holographically defined 3D PhCs. PhCs containing solid SU-8 features, layers of porous silicon (PSi) or emissive LaF3:Nd3+ nanocrystals, and silica colloids are formed. For the LaF3:Nd3+ layer, both enhancement (≈50%) and suppression (≈25%) of the spontaneous emission (λ ≈ 1.32 μm) could be realized by modifying the position of the photonic crystal stop band relative to the rare earth emission. Finite-difference time-domain simulations suggest the observed spontaneous emission modification is a result of Bragg mirror-like reflection, while the measured enhancement is likely caused by the spontaneous emission coupling to a defect mode. Via electrodeposition, this study demonstrates structural inversion of a low refractive index photonic crystal (photoresist-based) to a high (Cu2O) refractive index contrast photonic crystal in the presence of an embedded defect, providing an opportunity to enhance the light-matter interactions using a materials system with transparency in the visible.
KW - emission modification
KW - functional defects
KW - holographic photonic crystals
KW - material conversion
KW - transfer printing
UR - http://www.scopus.com/inward/record.url?scp=84973444163&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=84973444163&partnerID=8YFLogxK
U2 - 10.1002/adom.201600158
DO - 10.1002/adom.201600158
M3 - Article
AN - SCOPUS:84973444163
VL - 4
SP - 1533
EP - 1540
JO - Advanced Optical Materials
JF - Advanced Optical Materials
SN - 2195-1071
IS - 10
ER -